LrgpV1, Main, Exploration, bibRecord, 000B33

An experimental and kinetic investigation of premixed furan/oxygen/argon flames

Identifieur interne : 000B33 ( Main/Exploration ); précédent : 000B32; suivant : 000B34

An experimental and kinetic investigation of premixed furan/oxygen/argon flames

Auteurs : Zhenyu Tian [France, République populaire de Chine] ; Tao Yuan [République populaire de Chine] ; Rene Fournet [France] ; Pierre-Alexandre Glaude [France] ; Baptiste Sirjean [France] ; Frédérique Battin-Leclerc [France] ; Kuiwen Zhang [République populaire de Chine] ; Fei Qi [République populaire de Chine]

Source :

Combustion and flame [ 0010-2180 ] ; 2011.

RBID : PMC:3695461

English descriptors

mix :
- Premixed laminar flame Kinetic modeling Furan Tunable synchrotron VUV photoionization Molecular-beam mass spectrometry.

Abstract

The detailed chemical structures of three low-pressure (35 Torr) premixed laminar furan/oxygen/argon flames with equivalence ratios of 1.4, 1.8 and 2.2 have been investigated by using tunable synchrotron vacuum ultraviolet (VUV) photoionization and molecular-beam mass spectrometry. About 40 combustion species including hydrocarbons and oxygenated intermediates have been identified by measurements of photoionization efficiency spectra. Mole fraction profiles of the flame species including reactants, intermediates and products have been determined by scanning burner position with some selected photon energies near ionization thresholds. Flame temperatures have been measured by a Pt-6%Rh/Pt-30%Rh thermocouple. A new mechanism involving 206 species and 1368 reactions has been proposed whose predictions are in reasonable agreement with measured species profiles for the three investigated flames. Rate-of-production and sensitivity analyses have been performed to track the key reaction paths governing furan consumption for different equivalence ratios. Both experimental and modeling results indicate that few aromatics could be formed in these flames. Furthermore, the current model has been validated against previous pyrolysis results of the literature obtained behind shock waves and the agreement is reasonable as well.

Url:

DOI: 10.1016/j.combustflame.2010.12.022
PubMed: 23814311
PubMed Central: 3695461

Affiliations:

Le document en format XML

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<front><div type="abstract" xml:lang="en"><p id="P2">The detailed chemical structures of three low-pressure (35 Torr) premixed laminar furan/oxygen/argon flames with equivalence ratios of 1.4, 1.8 and 2.2 have been investigated by using tunable synchrotron vacuum ultraviolet (VUV) photoionization and molecular-beam mass spectrometry. About 40 combustion species including hydrocarbons and oxygenated intermediates have been identified by measurements of photoionization efficiency spectra. Mole fraction profiles of the flame species including reactants, intermediates and products have been determined by scanning burner position with some selected photon energies near ionization thresholds. Flame temperatures have been measured by a Pt-6%Rh/Pt-30%Rh thermocouple. A new mechanism involving 206 species and 1368 reactions has been proposed whose predictions are in reasonable agreement with measured species profiles for the three investigated flames. Rate-of-production and sensitivity analyses have been performed to track the key reaction paths governing furan consumption for different equivalence ratios. Both experimental and modeling results indicate that few aromatics could be formed in these flames. Furthermore, the current model has been validated against previous pyrolysis results of the literature obtained behind shock waves and the agreement is reasonable as well.</p>
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An experimental and kinetic investigation of premixed furan/oxygen/argon flames

An experimental and kinetic investigation of premixed furan/oxygen/argon flames

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